Piezoelectric materials generate an electric tension when mechanical stress is applied. This property enables the conversion of mechanical energy into electrical energy and vice-versa, making them of great interest for various applications. The most commonly used piezoelectric materials are inorganic crystals; however, they often have low mechanical flexibility, high production costs, and can be toxic due to the lead they may contain. A promising alternative is to exploit the piezoelectric properties of organic materials. In this talk, we will see how to induce and control a piezoelectric response in organic polymers.